By Lindsay M. Krall, Allison M. Macfarlane, Rodney C. Ewing
PNAS202111833_proof.pdf
Small modular reactors (SMRs; i.e., nuclear reactors that produce <300 MWelec each) have garnered attention because of claims of inherent safety features and reduced cost. However, remarkably few studies have analyzed the management and disposal of their nuclear waste streams. Here, we compare three distinct SMR designs to an 1,100-MWelec pressurized water reactor in terms of the energy-equivalent volume, (radio-)chemistry, decay heat, and fissile isotope composition of (notional) high-, intermediate-, and low- level waste streams. Results reveal that water-, molten salt–, and sodium-cooled SMR designs will increase the volume of nuclear waste in need of management and disposal by factors of 2 to 30. The excess waste volume is attributed to the use of neutron reflectors and/or of chemically reactive fuels and coolants in SMR designs. That said, volume is not the most important evaluation metric; rather, geologic repository performance is driven by the decay heat power and the (radio-)chemistry of spent nuclear fuel, for which SMRs provide no benefit. SMRs will not reduce the generation of geochemically mobile 129I, 99Tc, and 79Se fission products, which are important dose contributors for most repository designs. In addition, SMR spent fuel will contain relatively high concentra- tions of fissile nuclides, which will demand novel approaches to evaluating criticality dur- ing storage and disposal. Since waste stream properties are influenced by neutron leakage, a basic physical process that is enhanced in small reactor cores, SMRs will exacer- bate the challenges of nuclear waste management and disposal.
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